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[n]Cycloparaphenylene ([n]CPP) molecules have attracted broad interests due to their unique properties resulting from the distorted and strained aromatic hoop structures. In this work, we apply sub-nanometer resolved tip-enhanced Raman spectroscopy (TERS) to investigate the adsorption configurations and structural deformations of [12]CPP molecules on metal substrates with different crystallographic orientations. The TERS spectra for a [12]CPP molecule adsorbed on the isotropic Cu(10 surface are found to be essentially the same over the w
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