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We report on the electromagnetic properties of Co2+ substituted spinel MgCuZn ferrites developed via a facile molten salt synthesis (MSS) route. The choice of synthesis route in combination with cobalt substitution led to strong electromagnetic properties such as high saturation magnetization (i.e., 63 emu/g), high coercivity (17.86 gauss), and high initial permeability (273, which are beneficial for the multilayer chip inductor (MLCI) application. In a typical process, the planned ferrites were synthesized at 800 °C using sodium chlor