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We investigate the effects of an increase in the production of secondary electrons when a β-source commonly used in internal radionuclide therapy,67Cu, is radiolabelled to a Super-Paramagnetic Iron Oxide Nanoparticle (SPION), with specific emphasis on the role of SPION cluster size and geometry. A positive relationship is found between the degree to which the nanoparticles are clustered and the associated radio-enhancement effects, with cluster population size playing a major role, as well as SPION separation within a cluster and the dis
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