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Halloysite was first modified through vinyl functionalization, and subsequently polymerized with vinyl imidazole and 2-acrylamido-2-methylpropanesulfonic acid. Chlorosulfuric acid was used to transform the intertwined imidazole rings into acidic ionic liquids. UV-Vis spectroscopy and the Hammett equation indicated that the acid polyionic liquid's conjugation with halloysite resulted in an elevated acidity. A study into the catalyst's efficiency in producing 5-hydroxymethyl